I really cannot add anything to this thread. Everybody gave you great suggestions, and you already watched some of my favorite anime series (Cowboy Bebop, Evangelion, Gungrave, Hellsing). I just wanted to give my 2 cents about a couple of series already mentioned in this thread.
I loved Great Teacher Onizuka. As kupo said, it is much better than it sounds. I rarely had so much pure fun watching an anime, and most of the merit goes to Onizuka, one of the greatest and most original anime heroes/anti-heroes.
And as strange as it sounds, Azumanga Daioh is probably my favorite anime series. It's a bit Charles Schulz meets Japanese anime and manga... the world of AD is so delicate, poetic - at first, I thought it was "just" another cute anime, but it's so much more.
Oh, and I don't understand if you already watched it - but don't miss Trigun!!!
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